Impact of copper phthalocyanine structure on catalytic activity when incorporated into hierarchically porous carbon

Rina Adhikari,Molly Lockhart,Ambar Shrestha,Sabrina Curley, Ethan Hu,Kevin H. Shaughnessy, Michael K. Bowman,Martin G. Bakker

Molecular Catalysis（2022）

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摘要

•A one-pot reaction incorporates phthalocyanines into hierarchically porous carbon.•EPR spectroscopy shows some phthalocyanines survive heating to 500 °C.•Anionic phthalocyanine decomposes to large copper nanoparticles.•Cationic phthalocyanine decomposes to small copper nanoparticles.•Only the cationic phthalocyanine is catalytically active for cross-coupling reaction.

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关键词

Phthalocyanine,Hierarchically porous carbon,Sol-gel,One-pot,Copper nanoparticles

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