Unveiling Vibronic Coupling within the Q-bands of a Free-base Porphyrin

Vasilis Petropoulos,Mattia Russo,Pavel Rukin,Frank Quintela,Luca Moretti,Ana Moore,Thomas Moore,Devens Gust,Deborah Prezzi,Gregory Scholes,Elisa Molinari,Filippo Troiani,Giulio Cerullo,Carlo Rozzi,Margherita Maiuri

The International Conference on Ultrafast Phenomena (UP) 2022（2022）

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摘要

Multidimensional spectroscopies unveil the presence of vibronic coupling within the Q-states in a free-base porphyrin. High-frequency coupling and tuning modes drive the ultrafast internal conversion and track the excited state structural evolution.

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关键词

vibronic coupling,q-bands,free-base

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