TiO2 supported Pd nanoclusters with surface defects toward highly efficient hydrogenation of quinone to hydroquinone under mild conditions

Xiaoda Niu,Shuang Liu,Yong Men,Lin Li,Liangmin Xiong,Kailiang Guo,Junzhe Xu,Kunfeng Zhao,Ya Li,Wei An,Jinguo Wang

Molecular Catalysis（2022）

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摘要

•TiO2 supported Pd nanoclusters with surface defects (PdN/TiVo) were explored.•The properties of PdN/TiVo were analyzed and the coupled eutectic growth structure between Pd and TiO2 can be found.•PdN/TiVo catalysts exhibited considerably high yields and TOFs for the hydrogenation of TMBQ under mild conditions.•A mechanism for the synergistic catalytic hydrogenation of TMBQ over PdN/TiVo by metal Pd and oxygen vacancies was proposed.

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关键词

Pd catalyst,TiO2,Surface defects,Hydrogenation of quinones,Trimethylbenzoquinone

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