Plutonium reactive transport in fractured granite: Multi-species experiments and simulations

Xiaoying Zhang, Zheng Wang,Paul Reimus,Funing Ma,Mohamad Reza Soltanian,Baoshan Xing,Jianzheng Zang,Yu Wang,Zhenxue Dai

Water Research（2022）

引用 42|浏览5

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摘要

•The transport behaviors of Pu colloids, Pu(IV) and Pu(V-VI) were investigated.•The mobility is decreased from Pu colloid, Pu(V-VI) to Pu(IV).•Different models can describe the sorption of Pu in an unequivocally way.•Sorption rate constants of Pu tend to decrease with increasing time scales.

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关键词

Reactive transport,Sorption mechanism,Fractured rock,Pu species,Upscaling

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