Carbon-coated MoSe2/MXene heterostructures as active materials for high-performance Na+ batteries
MATERIALS TODAY COMMUNICATIONS(2022)
摘要
Despiting the technological promise and environmental friendliness of sodium-ion batteries (SIBs), relatively large sizes of Na-ions and moderate oxidation-reduction response slows down their wider-spread industrial implementation. To overcome this obstacle, we developed carbon-coated MoSe2/MXene heterostructures, in which MXene was covered on the MoSe2 particles and the loose carbon linked all the coated particles while providing porosity. The density-functional theory was used to understand the electronic structure of the carbon-coated MoSe2/MXene (MoSe2/Mo2CTx/C) and the mechanism of exchanging charge between MoSe2 and MXene. MoSe2/Mo2CTx/C as active anode material showed exceptional stability even after 2200 cycles in SIBs. Specif-ically, the capacities and retention rates observed for the batteries containing MoSe2/Mo2CTx/C and cycled at 0.5, 1, and 2 A g(-1) rates were equal to 652.2, 484.4, and 238.4 mAh g(-1) and 102.5%, 103.9%, and 86.3%, respectively. Thus, carbon-coated MoSe2/MXene can be utilized as active SIB anode materials.
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关键词
MXene, Sodium-ion batteries, MoSe 2, Active anode material
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