A novel radiation detector based on Gd2O3 doped organic semiconductor for the detection of γ and β-particles

E. Fukasawa,H. Miyata, E. Miyata, M. Katsumata, H. Sato, H. Ono, M. Watanabe, E. Saito, Y. Seino,A. Umeyama,M. Sato, M. Tamura,T. Suzuki

Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment(2022)

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摘要
A radiation detector that consists of a conducting polymer derived from an organic semiconductor material was developed. The motivation behind this study was to reduce the detector costs and to find a suitable alternative to large inorganic semiconductor detectors, which are difficult to fabricate. Herein, we report an unprecedented effort made to detect γ-particles using organic semiconductor, polyaniline, sensors. In addition, the novel organic semiconductor sensors also exhibited improved detection of β-particles compared with other conventional sensors. The material density of the sensor was increased to enhance the detection sensitivity. We focused on materials with high electron density and improved the γ and β-particle sensitivity by doping the material with gadolinium oxide (Gd2O3). When the Gd2O3 doped material was used in a hybrid organic–inorganic radiation detector, the detection sensitivity of the detector improved for γ-particles ejected from a 60Co source. Further, an attempt was made to fabricate sensors with improved β-particle sensitivity by adopting several approaches, including doping Gd2O3, using polyaniline with fine-tuned oxidation states, and modifying electrode designs. The target detector efficiency of 20% was achieved in the environment of a university laboratory, which is necessary to commercialize the organic radiation sensor.
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关键词
Organic semiconductor,Radiation detector,Detection efficiency
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