Metal-catalyzed C─H bond oxidation in the total synthesis of natural and unnatural products

Victor Camargo Stork Santana,Milena Cristina Vieira Fernandes, Isadora Cappuccelli, Ana Carolina Gonzales Richieri,Emilio Carlos de Lucca Júnior

Synthesis（2022）

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摘要

C―H bond oxidation has arisen as a powerful means for oxygen incorporation in organic molecules. Its use results in fast structural diversification and in a new way of thinking about retrosynthetic disconnections. In this review, we present the application of five metal-catalyzed methodologies for C(sp3)―H oxidation in the total synthesis of natural and unnatural products, covering the period of 2004–2022.

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关键词

C-H bond oxidation,catalysis,total synthesis,natural products,transition metals

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