A Stiffness Tunable Self-Healing Composite Comprising PDMS and Titanium Dioxide
ACS APPLIED POLYMER MATERIALS(2022)
摘要
It is a challenge to make artificial muscles with tunable stiffness capacities. The key is to develop a composite with tunable stiffness as well as self-healing properties and stretchability. In this work, we design a composite with amorphous TiO2 particles and poly(dimethylsiloxane) (PDMS) matrix cross-linked with metal-ligand interactions. The PDMS matrix enables the composite to have self-healing properties and excellent stretchability, while the interactions between the TiO2 particles can be enhanced by applying an electric field, which provides the composite with an electric field-controlled stiffness. The tunable storage modulus increased by 180% at 4 kV/mm. The stiffness of a simply supported beam increased by 10.8% at 6 kV with respect to that at 0 kV. Based on its tunable stiffness, self-healing properties and stretchability, this composite can mimic many functions of human muscles and has promising applications as an artificial muscle.
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关键词
self-healing,tunable stiffness,stretchability,electrorheological elastomer,artificial muscles
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