Gold-catalysed rearrangement of unconventional cyclopropane-tethered 1,5-enynes

Ruben Vicente,Eva Tudela,Miguel A. Rodriguez,Angel L. Suarez-Sobrino,Alfredo Ballesteros

CHEMICAL COMMUNICATIONS（2022）

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摘要

The synthesis of particular cyclopropane-tethered 1,5-enynes, namely 6-alkynyl-4-alkylidenebicyclo[3.1.0]hex-2-enes, enabled the discovery of unprecedented gold-catalyzed rearrangment to indenes. A computational study of the mechanism of this profound skeleton rearrangement is also disclosed.

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