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Cerium-oxo dusters for photocatalytic aerobic oxygenation of sulfides to sulfoxides

Xinjie Lv,Xiao-Li Zhao,Qixin Zhao,Qi Zheng,Weimin Xuan

DALTON TRANSACTIONS（2022）

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Abstract
Two cerium-oxo clusters (COCs) 1 and 2 are constructed by self-assembly of cerium ions and carboxylate ligands. Both clusters feature spherical structures resembling the key moiety of fluorite phase CeO2, and 1 exhibits high activity and selectivity for the photocatalytic aerobic oxygenation of sulfides to sulfoxides based on the switch between the Ce(IV/III) redox couple.
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photocatalytic aerobic oxygenation,sulfides,cerium-oxo
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