Bipolar charge transport in a robust hexacoordinate organosilane

Adam W. Earnhardt,Kevin M. Boyle,Tyler Adams,Michael G. Walter, Yizhou Wang,Yong Zhang,Adesola Adeyemi,Jon Merkert,Askhat N. Bimukhanov,Anuar A. Aldongarov,Colin D. McMillen,Thomas A. Schmedake

Journal of Organometallic Chemistry（2022）

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摘要

•Structurally characterized a hexacoordinate SiC4N2 complex with a distorted octahedral geometry.•Demonstrates bipolar charge transport in a thermally evaporated Si(pincer)2 complex.•Modeling indicates hole transfer involves a σ-delocalized HOMO.

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关键词

Hexacoordinate silicon,Organosilicon,Hypercoordinate,Bipolar charge transfer,Organic electronics

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