Impact of Wildfires on Meteorology and Air Quality (PM2.5 and O-3) over Western United States during September 2017

ATMOSPHERE(2022)

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摘要
In this study, we investigated the impact of wildfires on meteorology and air quality (PM2.5 and O-3) over the western United States during the September 2017 period. This is done by using Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) to simulate scenarios with wildfires (base case) and without wildfires (sensitivity case). Our analysis performed during the first half of September 2017 (when wildfire activity was more intense) reveals a reduction in modelled daytime average shortwave surface downward radiation especially in locations close to wildfires by up to 50 W m(-2), thus resulting in the reduction of the diurnal average surface temperature by up to 0.5 degrees C and the planetary boundary layer height by up to 50 m. These changes are mainly attributed to aerosol-meteorology feedbacks that affect radiation and clouds. The model results also show mostly enhancements for diurnally averaged cloud optical depth (COD) by up to 10 units in the northern domain due to the wildfire-related air quality. These changes occur mostly in response to aerosol-cloud interactions. Analysis of the impact of wildfires on chemical species shows large changes in daily mean PM2.5 concentrations (exceeding by 200 mu g m(-3) in locations close to wildfires). The 24 h average surface ozone mixing ratios also increase in response to wildfires by up to 15 ppbv. The results show that the changes in PM2.5 and ozone occur not just due to wildfire emissions directly but also in response to changes in meteorology, indicating the importance of including aerosol-meteorology feedbacks, especially during poor air quality events.
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关键词
wildfires, meteorology, air quality, WRF-Chem
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