Changes in Long-Term PM2.5 Pollution in the Urban and Suburban Areas of China's Three Largest Urban Agglomerations from 2000 to 2020

Particulate matter (PM2.5) is a significant public health concern in China, and the Chinese government has implemented a series of laws, policies, regulations, and standards to improve air quality. This study documents the changes in PM2.5 and evaluates the effects of industrial transformation and clean air policies on PM2.5 levels in urban and suburban areas of China's three largest urban agglomerations, Beijing-Tianjin-Hebei (BTH), the Yangtze River Delta (YRD), and the Pearl River Delta (PRD) based on a new degree of urbanization classification method. We used high-resolution PM2.5 concentration and population datasets to quantify the differences in PM2.5 concentrations in urban and suburban areas of these three urban agglomerations. From 2000 to 2020, the urban areas have expanded while the suburban areas have shrunk. PM2.5 concentrations in urban areas were approximately 32, 10, and 7 mu g/m(3) higher than those in suburban areas from 2000 to 2020 in BTH, YRD, and PRD, respectively. Since 2013, the PM2.5 concentrations in the urban regions of BTH, YRD, and PRD have declined at average annual rates of 7.30, 5.50, and 5.03 mu g/m(3)/year, respectively, while PM2.5 concentrations in suburban areas have declined at average annual rates of 3.11, 4.23 and 4.69 mu g/m(3)/year, respectively. By 2018, all of the urban and suburban areas of BTH, YRD, and PRD satisfied their specific targets in the Air Pollution and Control Action Plan. By 2020, the PM2.5 declines of BTH, YRD, and PRD exceeded the targets by two, three, and four times, respectively. However, the PM2.5 exposure risks in urban areas are 10-20 times higher than those in suburban areas. China will need to implement more robust air pollution mitigation policies to achieve the World Health Organization's Air Quality Guideline (WHO-AQG) and reduce long-term PM2.5 exposure health risks.