Modulating Photo- and Radioluminescence in Tb(III) Cluster-Based Metal-Organic Frameworks
ACS MATERIALS LETTERS(2022)
摘要
Luminescent metal-organic frameworks (MOFs) are of interest for sensing, theranostics, dosimetry, and other applications. The use of lanthanoids in MOF nodes allows for intrinsic metal-based luminescence. In this work, a facile route for modulating the photoluminescent and radioluminescent properties of Tb(III)-based MOFs is reported. By using Tb(III) cluster nodes as X-ray attenuators, and organic linkers with varying excited state energies as sensitizers, MOFs with metalbased, linker-based, and metal+linker-based photo- and radioluminescence are reported.
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关键词
metal–organic frameworks,radioluminescence,cluster-based
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