Nanomechanical Spectroscopy of 2D Materials.

Nano letters(2022)

Cited 4|Views29
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Abstract
We introduce a nanomechanical platform for fast and sensitive measurements of the spectrally resolved optical dielectric function of 2D materials. At the heart of our approach is a suspended 2D material integrated into a high silicon nitride nanomechanical resonator illuminated by a wavelength-tunable laser source. From the heating-related frequency shift of the resonator as well as its optical reflection measured as a function of photon energy, we obtain the real and imaginary parts of the dielectric function. Our measurements are unaffected by substrate-related screening and do not require any assumptions on the underling optical constants. This fast (τ ∼ 135 ns), sensitive (noise-equivalent power = ), and broadband (1.2-3.1 eV, extendable to UV-THz) method provides an attractive alternative to spectroscopic or ellipsometric characterization techniques.
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Key words
2D materials,NEMS,Nanomechanical resonators,silicon nitride,spectroscopy,transition metal dichalcogenides (TMDs)
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