Fluoreno[2,1-a]fluorene: an ortho-naphthoquinodimethane-based system with partial diradical character

Allison S. Hacker, Mauricio Pavano,James E. Wood,Hannah Hashimoto, Kyle M. D’Ambrosio,Conerd K. Frederickson,José L. Zafra,Carlos J. Gómez-García,Verònica Postils,Ashley Ringer McDonald,David Casanova,Derik K. Frantz,Juan Casado

Chemical Communications（2019）

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摘要

An ortho-naphtho diradical! Quinoidal forms in para- and meta-patterns lie at the extremes for closed-shell and diradical forms in fluorenofluorenes, respectively. ortho-Conjugation gives an intermediate case with partial diradical character.

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