Quantum coherence controls the charge separation in a prototypical artificial light harvesting system

Schramm H.,Cerullo G.,Maiuri M.,Brida D.,Molinari E.,Rubio A.,Spallanzani N.,Rozzi C. A.,Falke S.M., Christoffers J.,Lienau C.

EPJ Web of Conferences（2013）

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摘要

Ultrafast spectroscopy and quantum-dynamics simulations of an artificial supramolecular light-harvesting system — a supramolecular triad - provide strong evidence that the quantum-correlated wavelike motion of electrons and nuclei on a timescale of few tens of femtoseconds governs the ultrafast electronic charge transfer.

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关键词

charge separation,light

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