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Auxiliary‐Free Remote Dearomatizative Nitrenoid Transfer for Enantioselective Construction of Spirolactams

Bo‐Han Zhu,Wen‐Ting Guo,Qing Sun,Peng‐Cheng Qian,Long‐Wu Ye,Long Li

Advanced Synthesis and Catalysis（2022）

Cited 4|Views7
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Abstract
An Ir‐catalyzed remote dearomatizative amidation for the enantioselective construction of chiral spirolactams in 70–93% yield with 81–96% ee was developed. This protocol represented a more atom‐economical approach to chiral spirolactams via Ir‐catalyzed nitrenoid transfer without the introduction of a traceless O‐silyl achiral auxiliary.
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Key words
symmetric remote dearomatization,amidationn,nitrenoid transfer,chiral spirolactams
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