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Decoherence and Revival of Attosecond Charge Migration Driven by Non-adiabatic Dynamics

D. T. Matselyukh,V. Despré,N. V. Golubev,A. I. Kuleff,H.J. Wörner

Conference on Lasers and Electro-Optics（2021）

Cited 13|Views2
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Abstract
The attosecond quantum beat of an electronic state superposition was captured in SiH 4 using soft-X-Ray attosecond transient-absorption spectroscopy. Its decoherence and revival, induced by non-adiabatic vibrational dynamics, were reproduced using MCTDH calculations.
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Key words
attosecond charge migration,decoherence,non-adiabatic
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