Experimental Study of the Resonant Rovibrational Nonlinearity of CO2 and CO in the Mid-IR

2019 IEEE RESEARCH AND APPLICATIONS OF PHOTONICS IN DEFENSE CONFERENCE (RAPID)(2019)

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Abstract
We present time- and frequency-resolved measurements of self-focusing and self-defocusing of 4.3-4.8 μm Fe:ZnSe laser pulses tuned near rovibrational transitions of CO 2 And CO. We estimate the resonant nonlinearity of the air at 4.3 μm and discuss the novel nonlinear optics of simple molecules.
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Key words
Lasers,transition metal,Nonlinear optics,Kerr effect,Stark effect
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