Rh-Imiferrophos Complexes Catalyzed Asymmetric Hydrogenation Of Beta-Substituted Alpha,Beta-Unsaturated Phosphonates
CHINESE JOURNAL OF CATALYSIS（2014）
Abstract
A series of chiral ferrocenyl diphosphine ligands (ImiFerroPhos ligands) has been applied to the hydrogenation of beta-substituted alpha,beta-unsaturated phosphonates to generate a range of optically active beta-substituted alkylphosphonates in good yields with good enantioselectivity (up to 92% ee) under mild reaction conditions. (C) 2014, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
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Key words
beta-Substituted alpha,beta-unsaturated phosphonate,Asymmetric catalytic hydrogenation,ImiFerroPhos ligands,Rhodium (II) complex,Chiral beta-substituted alkylphosphonate
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