A sustainable and green route to furan-2,5-dicarboxylic acid by direct carboxylation of 2-furoic acid and CO2
Journal of CO2 Utilization（2021）
Abstract
•Carboxylation involved hydrogen abstraction in 2-furoate and electrophilic addition of CO2.•Hydrogen abstraction of furan ring was rate-determining.•Selective generation of 2,5-FDCA depended on hydrogen abstraction step and molecular features of 2-furoate.
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Key words
Chemical utilization of CO2,Synthesis of 2,5-furandicarboxylic acid,Direct carboxylation,Lignocellulose bio-based compound
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