Coexistence of ferromagnetism and spin-orbit coupling by incorporation of platinum in two-dimensional VSe$_2$

E. Vélez-Fort, A. Hallal, R. Sant,T. Guillet, K. Abdukayumov,A. Marty, C. Vergnaud, J. -F. Jacquot, D. Jalabert,J. Fujii,I. Vobornik,J. Rault,N. B. Brookes,D. Longo, P. Ohresser, A. Ouerghi,J. -Y. Veuillen, P. Mallet, H. Boukari,H. Okuno,M. Chshiev, F. Bonell,M. Jamet

arxiv(2021)

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摘要
We report on a novel material, namely two-dimensional (2D) V$_{1-x}$Pt$_x$Se$_2$ alloy, exhibiting simultaneously ferromagnetic order and Rashba spin-orbit coupling. While ferromagnetism is absent in 1T-VSe$_2$ due to the competition with the charge density wave phase, we demonstrate theoretically and experimentally that the substitution of vanadium by platinum in VSe$_2$ (10-50 %) to form an homogeneous 2D alloy restores ferromagnetic order with Curie temperatures of 6 K for 5 monolayers and 25 K for one monolayer of V$_{0.65}$Pt$_{0.35}$Se$_2$. Moreover, the presence of platinum atoms gives rise to Rashba spin-orbit coupling in (V,Pt)Se$_2$ providing an original platform to study the interplay between ferromagnetism and spin-orbit coupling in the 2D limit.
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