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Skeleton-Sn anchoring isolated Pt site to confine subnanometric clusters within *BEA topology

Yue Ma,Xiao Chen,Yejun Guan,Hao Xu,Jiangwei Zhang,Jingang Jiang,Li Chen,Teng Xue,Qingsong Xue,Fei Wei,Peng Wu

Journal of Catalysis（2021）

Cited 25|Views15
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Abstract
•Confined subnanometric Pt clusters within Sn-Beta were synthesized by impregnation-reduction.•(Si-O)3(H2O)2Sn(IV)-(O)-[PtCl5]− species sever as the key precursors of Pt clusters less than 1 nm.•Framework Sn coordinated Pt clusters show good stability in PDH at 500 °C.
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Key words
Subnanometric clusters,Framework-Sn,Anchoring effect,Excellent stability,Ultra-high selectivity
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