Dissecting the interfaces of MOF-coated CdS on synergized charge transfer for enhanced photocatalytic CO2 reduction

Qiaoqiao Mu,Yanhui Su,Zhihe Wei, Hao Sun,Yuebin Lian, Yuyi Dong,Pengwei Qi,Zhao Deng,Yang Peng

Journal of Catalysis（2021）

引用 53|浏览7

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摘要

•Core-shell structured CdS@Co(BDC) nanorods are successfully synthesized.•Co(BDC) bridges the heterogeneous photosensitizer and molecular co-catalyst.•Catalytic performance is ranked atop metal sulfide photocatalysts reported so far.•Electron transfer at interfaces of photocatalytic system are explicitly illustrated.•The catalytic mechanism is elucidated engaging LMCT and PCET processes.

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关键词

Photocatalysis,CO2 reduction reactions,Metal organic frameworks,CdS

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