Atomic Layer Deposition of Yttrium Iron Garnet Thin Films for 3D Magnetic Structures
arxiv(2021)
摘要
A wide variety of new phenomena such as novel magnetization configurations
have been predicted to occur in three dimensional magnetic nanostructures.
However, the fabrication of such structures is often challenging due to the
specific shapes required, such as magnetic tubes and spirals. Furthermore, the
materials currently used to assemble these structures are predominantly
magnetic metals that do not allow to study the magnetic response of the system
separately from the electronic one. In the field of spintronics, the
prototypical material used for such experiments is the ferrimagnetic insulator
yttrium iron garnet (Y_3Fe_5O_12, YIG). YIG is one of the best
materials especially for magnonic studies due to its low Gilbert damping. Here,
we report the first successful fabrication of YIG thin films via atomic layer
deposition. To that end we utilize a supercycle approach based on the
combination of sub-nanometer thin layers of the binary systems Fe_2O_3 and
Y_2O_3 in the correct atomic ratio on Y_3Al_5O_12 substrates with a
subsequent annealing step. Our process is robust against typical growth-related
deviations, ensuring a good reproducibility. The ALD-YIG thin films exhibit a
good crystalline quality as well as magnetic properties comparable to other
deposition techniques. One of the outstanding characteristics of atomic layer
deposition is its ability to conformally coat arbitrarily-shaped substrates.
ALD hence is the ideal deposition technique to grant an extensive freedom in
choosing the shape of the magnetic system. The atomic layer deposition of YIG
enables the fabrication of novel three dimensional magnetic nanostructures,
which in turn can be utilized for experimentally investigating the phenomena
predicted in those structures.
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关键词
magnetic structures,thin films
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