Magnetic‐Field‐Controlled Quantum Critical Points in the Triangular Antiferromagnetic Cs2CuCl4‐xBrx Mixed System
Annalen der Physik(2020)
摘要
The triangular antiferromagnetic Cs2CuCl4‐xBrx mixed system is studied by neutron single‐crystal diffraction in magnetic field. It shows a rich magnetic phase diagram consisting of four regimes depending on the Br concentration and is characterized by different exchange coupling mechanisms. For the investigated compositions from regime I (0 \u003c x ≤ 1.5), a critical magnetic field Bc is found for a Br concentration x = 0.8 at Bc = 8.10(1) T and for x = 1.1 at Bc = 7.73(1) T and from regime IV (3.2 \u003c x \u003c 4) for x = 3.3 at Bc = 0.99(3) T. For magnetic fields larger than the respective Bc, magnetic superlattice reflections of these compounds are not found. The incommensurate magnetic wave vector q = (0, 0.470, 0) appears below the ordering temperature TN = 0.51(1) K for Cs2CuCl3.2Br0.8, and q = (0, 0.418, 0) below TN = 1.00(6) K for Cs2CuCl0.3Br3.7. Neutron diffraction experiments at around 60 mK for x = 3.7 in a magnetic field show the critical magnetic field at Bc = 7.94(16) T and the formation of the second magnetic phase at around 8.5 T depending on the temperature. Inelastic neutron scattering experiments for the compound from regime III (2 \u003c x ≤ 3.2) with x = 2.2 show dynamical correlations at a temperature around 50 mK giving evidence for a spin liquid phase.
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关键词
Cs2CuCl4-xBrx mixed system, magnetic order
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