Preparation of Cu single atoms on N-doped carbon materials with supercritical CO2 deposition

The Journal of Supercritical Fluids(2021)

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摘要
•Cu single-atom on N-doped carbon materials by supercritical CO2 deposition.•N-doped carbon is a mesoporous material with a high surface area of 1301 m2/g.•Atomically dispersed metal atoms were prepared without further post-treatment.•AC-HAADF-STEM confirms that Cu atoms are equally dispersed over the NC support.•Cu-NC shows excellent performance in oxidation of benzyl alcohol to benzaldehyde.
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关键词
SACs,SCFD,NC,Cu-NC,O*,TBHP
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