Pressure Influence On The Valence And Magnetic State Of Yb Ions In Noncentrosymmetric Heavy-Fermion Ybnic2

PHYSICAL REVIEW B(2021)

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摘要
We present studies of neutron diffraction, electrical resistivity, magnetic susceptibility, magnetization, and specific heat of noncentrosymmetric YbNiC2. At normal pressure, YbNiC2 is a moderate heavy-fermion compound with Kondo lattice. At 16 K we observe an anomaly in the temperature dependence of specific heat which is ascribed to an abrupt valence change of Yb ions. At pressures above 7 GPa, the valence change and the Kondo lattice state are suppressed, and near a temperature of 10 K we detect the appearance of magnetic order. Above 5 GPa, the temperature dependence of the resistivity behaves similarly to other compounds of the CeNiC2-type family, indicating the formation of charge density waves. This is attributed to the nesting properties of the Fermi surface (FS) found within the density functional theory + dynamical mean field theory treatment. Our ab initio calculations also show that the valence of Yb in YbNiC2 at normal conditions is 2.85, which increases with temperature and pressure. The FS of YbNiC2 is anisotropic in shape in comparison with the 3D surface of YbCoC2.
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关键词
yb ions,magnetic state,heavy-fermion
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