Systematic detection of local CH 4 emissions anomalies combining satellite measurements and high-resolution forecasts

Atmospheric Chemistry and Physics(2020)

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摘要
Abstract. In this study we present a novel monitoring methodology to detect local CH4 concentration anomalies worldwide that are related to rapidly changing anthropogenic emissions that significantly contribute to the CH4 atmospheric budget. The method uses high resolution (7 km × 7 km) retrievals of total column CH4 from the Tropospheric Monitoring Instrument (TROPOMI) onboard the Sentinel 5 Precursor satellite. Observations are combined with high resolution CH4 forecasts (~ 9 km) produced by the Copernicus Atmosphere Monitoring Service (CAMS) to provide departures (observations minus forecasts) close to the native satellite resolution at appropriate time. Investigating the departures is an effective way to link satellite measurements and emission inventory data in a quantitative manner. We perform filtering on the departures to remove the large-scale biases on both forecasts and satellite observations. We then use a simple classification on the filtered departures to detect anomalies and plumes coming from CAMS emissions that are missing (e.g. pipeline or facility leaks), under-reported or over-reported (e.g. depleted drilling fields). Additionally, the classification helps to detect local satellite retrieval errors due to land surface albedo issues.
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