Simulating exciton migration and annihilation dynamics in higher order spectroscopies of a molecular trimer
EPJ Web of Conferences(2019)
摘要
We present simulations of 3rd and 5th order multidimensional time-dependent signals of a molecular trimer. The developed model allows for the simulation of both signal types within one theoretical framework. We therefore extended standard Redfield theory of exciton migration by a new term to include the process of exciton-exciton annihilation.
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