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Direct observation of structural dynamics upon photo-excitation in a spin crossover crystal with femtosecond electron diffraction

Yifeng Jiang,Lai Chung Liu,Henrike M. Mueller-Werkmeister,Cheng Lu,Dongfang Zhang,Ryan L. Field,Antoine Sarracini,Gustavo Moriena,Eric Collet,R. J. Dwayne Miller

EPJ Web of Conferences（2019）

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Abstract
Photoinduced spin transitions are studied by femtosecond electron diffraction to understand ultrafast structural dynamics associated with intersystem crossing. The results indicate the structural reorganization occurs within 2.3 ps, as the metal-ligand bond distribution narrows during intramolecular vibrational energy redistribution.
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Key words
spin crossover crystal,electron diffraction,structural dynamics,photo-excitation
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