Single-Ni-atom catalyzes aqueous phase electrochemical reductive dechlorination reaction
Applied Catalysis B: Environmental（2020）
Abstract
•Atomically dispersed Ni (A-Ni-NG) electrocatalyst was developed for dechlorination.•A-Ni-NG exhibited highest activities to dechlorination of chloroacetic acids (CAAs).•High activity of A-Ni-NG stems from its specific interactions with intermediate.•The Cl atoms in CAAs are eliminated sequentially through a direct mechanism.•Electron transfer step occurs in a stepwise manner with breaking C–Cl bond.
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Key words
Reductive dechlorination,Chloroacetic acids,Single atom catalyst,Dechlorination pathway,Catalytic mechanism
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