Experimental demonstration of pressurized chemical looping combustion in an internally circulating reactor for power production with integrated CO2 capture

Chemical Engineering Journal(2020)

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摘要
•Internally circulating reactor (ICR) was demonstrated for chemical looping combustion at pressurized condition up to 6.0 bar.•The ICR is proposed and design to simplify the operation and scale-up of chemical looping processes at high-pressure.•The solids circulation rate was found to increase with increasing the operating pressure at a constant fluidization velocity.•CO2 capture efficiency and purity up to 97% was achieved, and found to be insensitive to the operating pressure.•Autothermal high-pressure CLC operation using ICR was achieved.
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关键词
Chemical looping combustion,High pressure operation,Internally circulating reactor,Fluidized-bed, CO2 capture,Correlation for solids circulation rate
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