Ultrafast, Zero-Bias, Graphene Photodetectors With Polymeric Gate Dielectric On Passive Photonic Waveguides

ACS NANO(2020)

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摘要
We report compact, scalable, high-performance, waveguide integrated graphene-based photodetectors (GPDs) for telecom and datacom applications, not affected by dark current. To exploit the photothermoelectric (PTE) effect, our devices rely on a graphene/polymer/graphene stack with static top split gates. The polymeric dielectric, poly(vinyl alcohol) (PVA), allows us to preserve graphene quality and to generate a controllable p-n junction. Both graphene layers are fabricated using aligned single-crystal graphene arrays grown by chemical vapor deposition. The use of PVA yields a low charge inhomogeneity similar to 8 X 10(10) cm(-2) at the charge neutrality point, and a large Seebeck coefficient similar to 140 mu V K-1, enhancing the PTE effect. Our devices are the fastest GPDs operating with zero dark current, showing a flat frequency response up to 67 GHz without roll-off. This performance is achieved on a passive, low-cost, photonic platform, and does not rely on nanoscale plasmonic structures. This, combined with scalability and ease of integration, makes our GPDs a promising building block for next-generation optical communication devices.
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关键词
graphene, photodetectors, photothermoelectric effect, polymeric dielectric, integrated photonics, optoelectronics
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