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Pd model catalysts: Effect of aging environment and lean redispersion

Jason A. Lupescu,Johannes W. Schwank,Kevin A. Dahlberg,Chang Yup Seo,Galen B. Fisher,Sabrina L. Peczonczyk,Kevin Rhodes,Mark J. Jagner,Larry P. Haack

Applied Catalysis B: Environmental（2016）

Cited 33|Views4
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Abstract
•Different aging environments at 700°C lead to different catalyst structures.•The aging environment severity ranking was: redox>rich-only>>lean-only.•Aged catalysts exhibited metal oxidation effects and support/additive interactions.•Exposure of aged catalysts to 700°C air improved activity despite low Pd dispersion.•Multiple 700°C air treatments were needed to restore Pd dispersion on CZO.
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Key words
Palladium,Redispersion,TWC,Regeneration
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