The Ginninderra CH 4 and CO 2 release experiment : An evaluation of gas detection and quanti fi cation techniques

semanticscholar(2018)

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摘要
A methane (CH4) and carbon dioxide (CO2) release experiment was held from April to June 2015 at the Ginninderra Controlled Release Facility in Canberra, Australia. The experiment provided an opportunity to compare different emission quantification techniques against a simulated CH4 and CO2 point source release, where the actual release rates were unknown to the participants. Eight quantification techniques were assessed: three tracer ratio techniques (two mobile); backwards Lagrangian stochastic modelling; forwards Lagrangian stochastic modelling; Lagrangian stochastic (LS) footprint modelling; atmospheric tomography using point and using integrated line sensors. The majority of CH4 estimates were within 20% of the actual CH4 release rate (5.8 g/min), with the tracer ratio technique providing the closest estimate to both the CH4 and CO2 release rates (100 g/min). Once the release rate was known, the majority of revised estimates were within 10% of the actual release rate. The study illustrates the power of measuring the emission rate using multiple simultaneous methods and obtaining an ensemble median or mean. An ensemble approach to estimating the CH4 emission rate proved successful with the ensemble median estimate within 16% for the actual release rate for the blind release experiment and within 2% once the release rate was known. The release also provided an opportunity to assess the effectiveness of stationary andmobile ground and aerial CH4 detection technologies. Sensor detection limits and sampling rates were found to be significant limitations for CH4 and CO2 detection. A hyperspectral imager’s capacity to image the CH4 release from 100m, and a Boreal CH4 laser sensor’s ability to track moving targets suggest the future possibility to map gas plumes using a single laser and mobile aerial reflector. https://doi.org/10.1016/j.ijggc.2017.11.018 Received 4 August 2017; Received in revised form 14 November 2017; Accepted 18 November 2017 ⁎ Corresponding author at: Geoscience Australia, Canberra, Australia. E-mail address: andrew.feitz@ga.gov.au (A. Feitz). International Journal of Greenhouse Gas Control 70 (2018) 202–224 Available online 15 March 2018 1750-5836/ Crown Copyright © 2017 Published by Elsevier Ltd. This is an open access article under the CC BY license (http://creativecommons.org/licenses/BY/4.0/). T
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