Mechanism of thermal decomposition of HFO-1234ze(E) under supercritical fluid conditions
The Journal of Supercritical Fluids(2020)
Abstract
•HFO-1234ze(E) decomposition mechanisms were investigated.•Under mild conditions, HFO-1234ze(E) decomposed to C2C3 HFC gases.•Under harsh conditions, liquids, coke and long-chain HFC gases were formed.•HF elimination and HF addition were the main decomposition mechanisms.
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Key words
Supercritical organic Rankine cycle,HFO-1234ze(E),Thermal decomposition,Density functional theory,HF addition and elimination
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