Insights into the Role of Cation Vacancy for Significantly Enhanced Electrochemical Nitrogen Reduction

Xiaohui Yang,Faling Ling,Jinfeng Su,Xiangrong Zi,Han Zhang,Huijuan Zhang,Jian Li,Miao Zhou,Yu Wang

Applied Catalysis B: Environmental（2020）

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摘要

The introduction of Mo vacancies in MoN can regulate its electronic properties, shift the potential-determining step (PDS) of NRR and induce the reduction of PDS barrier height from 1.40 to 0.61 eV, significantly enhancing NRR performance.

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关键词

Mo vacancies MoN nanocrystal,Electrocatalysis,Artificial N2 fixation,Mars-van krevelen mechanism,NH3

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