Sulfated ZrO2 supported CoMo sulfide catalyst by surface exsolution for enhanced hydrodeoxygenation of lignin-derived ethers to aromatics
Fuel（2020）
Abstract
•Bifunctional CoMo sulfide-sulfated ZrO2 are prepared by in situ exsolution method.•CoMo-sZr(exs) catalyst shows a high HDO activity and high aromatics selectivity.•Appropriate sulfide-support interaction results in a uniformly MoS2 dispersion.•Acid sites facilitate oxy-compound adsorption and C-O bond cleavage.
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Key words
In situ exsolution,CoMo sulfide,Sulfated ZrO2,Lignin-derived ethers,Selective C–O cleavage,Hydrodeoxygenation
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