Two-Photon Absorption In A Two-Level System Enabled By Noise

We address the textbook problem of dynamics of a spin placed in a dc magnetic field and subjected to an ac drive. If the drive is polarized in the plane perpendicular to the dc field, then the drive photons are resonantly absorbed when the spacing between the Zeeman levels is close to the photon energy. This is the only resonance when the drive is circularly polarized. For a linearly polarized drive, additional resonances corresponding to absorption of three, five, and multiple odd numbers of photons is possible. Interaction with the environment causes the broadening of the absorption lines. We demonstrate that the interaction with environment enables the forbidden two-photon absorption. We adopt a model of the environment in the form of random telegraph noise produced by a single fluctuator. As a result of the synchronous time fluctuations of different components of the random field, the shape of the two-photon absorption line is non-Lorentzian and depends dramatically on the drive amplitude. This shape is a monotonic curve at strong drive, while, at weak drive, it develops a two-peak structure reminiscent of an induced transparency on resonance.