Optically Pumped Lasing Of Segregated Quasi-2d Perovskite Microcrystals In Vertical Microcavity At Room Temperature

Quasi-2D Ruddlesden-Popper perovskites possess a tailorable quantum well structure and outstanding optical properties. Herein, we study their diverse phase-separation phenomena and the resulting microcrystals (similar to 1 mu m), which have evidently enhanced photoluminescence. Lasing based on these microcrystals in a vertical single-mode optical microcavity has also been achieved, featuring a low threshold of similar to 500.0 mu J/cm(2) pumped by a nanosecond pulsed laser (355 nm, pulse width 8 ns, 1 kHz). This work makes the quasi-2D perovskite microcrystals potential candidates to be gain materials for continuous wave lasing.