Ultra-fast fabrication of bulk ZrNiSn thermoelectric material through self-propagating high-temperature synthesis combined with in-situ quick pressing
Scripta Materialia(2019)
Abstract
The conventional fabrication of bulk thermoelectric materials usually involves time and energy consuming steps including melting, annealing and sintering et al, which restricts the large-scale application. Herein, high thermoelectric performance ZrNiSn bulks were synthesized by one step self-propagating high-temperature synthesis combining with in-situ quick pressing (SHS-QP). The correlation among SHS process, QP process and the critical pressure, is systematically investigated. The reduced grain size due to non-equilibrium feature of SHS-QP leads to a significant reduction in the thermal conductivity and a high figure of merit ZT ~ 0.7.
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Key words
Thermoelectric materials,SHS,Half-Heusler
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