Effect of composition and preparation of supported MoO3 catalysts for anisole hydrodeoxygenation

Chanakya Ranga,Rune Lødeng,Vaios I. Alexiadis,Tapas Rajkhowa,Hilde Bjørkan,Svatopluk Chytil,Ingeborg H. Svenum,John Walmsley,Christophe Detavernier,Hilde Poelman,Pascal Van Der Voort,Joris W. Thybaut

Chemical Engineering Journal（2018）

Cited 77|Views7

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Abstract

•Crystallinity of MoO3 and Zr(MoO4)2 increases significantly with Mo loading.•H2/CH4 (80/20 vol%) treatment at 550 and 700 °C induces Mo5+ and Mo4+ formation.•Mo5+ species are particularly active and stable during anisole HDO.•Hydrodeoxygenation prevails over hydrogenation during anisole conversion over Mo.

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Key words

Bio-oil,Hydrodeoxygenation,Gas phase,Anisole,Molybdenum oxide,Reaction pathway

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