Highly selective catalytic combustion of acrylonitrile towards nitrogen over Cu-modified zeolites
Catalysis Today(2019)
摘要
•Cu-exchanged zeolites achieving both high C2H3CN conversion and N2 selectivity.•Oxidation/hydrolysis mechanism was proposed on experimental and theoretical approaches.•Change transfer during nitrile elimination was analyzed by Mulliken method.
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关键词
Acrylonitrile (C2H3CN),Selective catalytic combustion (SCC) mechanism,Cu-ZSM-5,DFT,Mulliken charge transfer
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