Mild-acid-assisted thermal or hydrothermal dealumination of zeolite beta, its regulation to Al distribution and catalytic cracking performance to hydrocarbons
Journal of Catalysis(2018)
摘要
•Dilute HCl combined with steaming or calcination removed ∼70% Al of zeolite β.•Combined dealumination was more versatile than single treatment.•Acid steaming removed Al on T2, T5, T6, and T7 sites and drove poly-EFAL to external surface.•Acid calcination resulted in a more homogeneous Al distribution in zeolite β structure.•Acid calcination caused stronger B acidity and higher B acid density than acid steaming.
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关键词
Zeolite beta,Dealumination,Al distribution,Acidity,Catalytic cracking
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