Influence of Zr on the performance of Mg-Al catalysts via hydrotalcite-like precursors for the synthesis of glycerol carbonate from urea and glycerol
Applied Catalysis A: General(2018)
Abstract
•Tunable acidic-basic property of mesoporous Mg-Al-Zr mixed oxides was obtained.•The role of acidic and basic sites was clarified in overall reaction as well as in every comprising reaction pathway.•A well-balanced acidic-basic property was important for the catalyst to obtain high GLC yield with good selectivity.•A higher GLC yield of 87.8% with 90.8% excellent selectivity could be achieved.
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Key words
Glycerol,Glycerol carbonate,Urea,Hydrotalcite-like,Acidic-basic property
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