Oxidative dehydrogenation of ethane using MoO3/Fe2O3 catalysts in a cyclic redox mode
Catalysis Today（2018）
Abstract
•MoO3/Fe2O3 core-shell redox catalysts prepared.•Calcined catalysts have surface layers comprising Fe2(MoO4)3 and MoO3.•Core-shell catalysts exhibit enhanced ethane CL-ODH performance.•Mixed Mo-Fe oxide shell suppresses combustion and increases ODH activity.
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Key words
Oxidative dehydrogenation,Chemical looping,Molybdenum oxide,Iron oxide,X-ray photoelectron spectroscopy,Diffuse reflectance infrared Fourier transform spectroscopy,Temperature-programmed reduction
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