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Separating and probing tautomers of protonated nucleobases using differential mobility spectrometry

Ahdia Anwar,Jarrod Psutka,Stephen W.C. Walker,Thorsten Dieckmann, John S. Janizewski,J. Larry Campbell,W. Scott Hopkins

International Journal of Mass Spectrometry（2018）

Cited 29|Views16
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Abstract
•Protonated nucleobase tautomers are separated by DMS and probed by MS.•Tautomer populations are tuned by selective fragmentation.•DMS signals are distinguished by monitoring ion signal as a function of declustering potential.
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Key words
Nucleobases,Differential mobility spectrometry,Hydrogen-deuterium exchange,Enhanced product ion,Density functional theory,Coupled cluster theory,Clusters
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