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Significant electron transfer in heme catalysis: The case of chlorite dismutase

Jing-Xuan Su,Shi-Lu Chen

Journal of Catalysis（2017）

Cited 13|Views4
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Abstract
•A transition state for electron transfer in heme catalysis has been characterized.•Cld-catalyzed PAA reaction proceeds via homolytic OO bond cleavage followed by ET.•Compounds II and I are successively formed during the PAA reaction.•Different binding modes for PAA do not change the mechanism significantly.•A heme enzyme may employ different mechanisms for different substrates.
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Key words
Chlorite dismutase,Density functional calculations,Electron transfer,Heme proteins,Peracetic acid
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